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Different timescales during ultrafast stilbene isomerization in the gas and liquid phases revealed using time-resolved photoelectron spectroscopy

Nature Chemistry, Published online: 11 August 2022; doi:10.1038/s41557-022-01012-0The influence that liquid environments have on the ultrafast excited-state dynamics of molecules is poorly understood. Using time-resolved photoelectron spectroscopy, the dynamics of the photoisomerization of stilbene in the gas and liquid phases have now been shown to...

Filling of a water-free void explains the allosteric regulation of the β<sub>1</sub>-adrenergic receptor by cholesterol

Nature Chemistry, Published online: 11 August 2022; doi:10.1038/s41557-022-01009-9The β1-adrenergic receptor (β1AR) contains empty cavities in its preactive conformation, which disappear in the active one. Now, using X-ray crystallography of xenon-derivatized β1AR crystals, a cavity has been shown to be in contact with the cholesterol-binding pocket....

Standardized excitable elements for scalable engineering of far-from-equilibrium chemical networks

The ribosome stabilizes partially folded intermediates of a nascent multi-domain protein

Synthesis of a low-valent Al<sub>4</sub><sup>+</sup> cluster cation salt

Standardized excitable elements for scalable engineering of far-from-equilibrium chemical networks

Nature Chemistry, Published online: 04 August 2022; doi:10.1038/s41557-022-01001-3Synthetic chemical networks with far-from-equilibrium dynamics akin to genetic regulatory networks in living cells could precisely regulate the kinetics of chemical synthesis or self-assembly. Now standardized excitable chemical regulatory elements, termed genelets, that...

The ribosome stabilizes partially folded intermediates of a nascent multi-domain protein

Nature Chemistry, Published online: 04 August 2022; doi:10.1038/s41557-022-01004-0Most proteins must fold co-translationally on the ribosome to adopt biologically active conformations, yet structural, mechanistic descriptions are lacking. Using 19F NMR spectroscopy to study a nascent multi-domain protein has now enabled the identification of two co-translational...

Synthesis of a low-valent Al<sub>4</sub><sup>+</sup> cluster cation salt

Nature Chemistry, Published online: 04 August 2022; doi:10.1038/s41557-022-01000-4Although neutral and anionic low-valent aluminium complexes are widespread, their cationic counterparts have remained rare. Now, a salt of [Al(AlCp*)3]+ featuring a formal low-valent Al+ cation has been isolated that dimerizes in concentrated solutions and the solid state,...

Photochemical single-step synthesis of β-amino acid derivatives from alkenes and (hetero)arenes

Ambient-light-induced intermolecular Coulombic decay in unbound pyridine monomers

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