Wiley Online Library : Advanced Energy Materials
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Regulating Ion Diffusion and Stability in Amorphous Thiosilicate‐Based Solid Electrolytes Through Edge‐Sharing Local Structures

A novel amorphous SSE 5Li2S-3SiS2 (mol %) with a high ionic conductivity of 1.2 mS cm−1 is reported. The silicon and sulfur atoms in the edge-sharing Si2S6 4− are less attracted to lithium compared to the SiS4 4− anion, which is expected to facilitate the lithium ions conduction in SSEs. More importantly, the Si2S6 4− indicates better stability...

Mon Jun 17, 2024 12:18
Prussian Blue Analogues for Aqueous Sodium‐Ion Batteries: Progress and Commercialization Assessment

Aqueous sodium-ion batteries (ASIBs) are a compelling option for energy storage systems. The advantages and challenges of Prussian blue analogues as cathode materials for ASIBs are highlighted. Modification strategies at the material level, as well as the design of the full cells, are discussed in depth. The prospect of commercialization is discussed,...

Mon Jun 17, 2024 12:18
Lithium Battery‐Powered Extreme Environments Exploring: Principle, Progress, and Perspective

This comprehensive review delves into the fundamental understanding of the service behavior of lithium batteries in extreme external physical fields. It focuses on elucidating the unique physicochemical principle and the underlying mechanisms of thermodynamic and kinetic processes that arise from these external extreme forces. Finally, the potential...

Mon Jun 17, 2024 12:18
Solvation Barrier Remodeling‐Dictated Fast‐Kinetics Top–Down Zn Stripping/Plating in Water‐Lean Organic Electrolytes

A chelation-induced solvation barrier remodeling strategy is initiated toward fast-kinetics “top–down” Zn stripping/plating in original Zn2+-free water-lean organic electrolytes (WLOE) for durable Zn batteries. The intervention of multidentate chelant (2-methoxyethylamine, MEA) in WLOE greatly lowers the solvation reorganization energy of in situ...

Mon Jun 17, 2024 12:18
Homogeneous In‐Plane Lattice Strain Enabling d‐Band Center Modulation and Efficient d–π Interaction for an Ag2Mo2O7 Cathode Catalyst With Ultralong Cycle Life in Li‐O2 Batteries

The homogeneous in-plane distortion of Ag2Mo2O7 leads to d-band center optimization and the spatial and energy overlap of Ag dxz and O2 anti-bonding π* orbitals, achieving highly efficient catalytic activity and rapid ORR/OER kinetics with an ultralong cycle life of 817 cycles at a current density of 500 mA g‒1 in LOBs. Abstract Although...

Sat Jun 15, 2024 11:37
Ternary Metal Sulfides as Electrode Materials for Na/K‐Ion Batteries and Electrochemical Supercapacitor: Advances/Challenges and Prospects

Ternary metal sulfides (TMSs) show potential as electrode materials for rechargeable batteries and supercapacitors (SCs). However, their real-world application faces challenges. This review discusses strategies for enhancing electrochemical activity through tailored nanostructures, backed by a comprehensive literature survey of recent advancements....

Sat Jun 15, 2024 11:37

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